Unless you want to add new stock, the low pH is likely not an issue (given fish species mentioned)
Rather than a larger single water change, I’d suggest moving to twice weekly 50l water changes and see how that impacts your pH ... if you want to raise pH in this tank, it should be done slowly, steadily
I’d plan on bringing the pH up to 6 over several weeks (while fish may manage a faster rise in pH, the shift will likely impact the environment as a whole) - and likely would not aim for pH above 6-6.4 (though again this depends on your intended goals)
Note my tap water is now reported as pH 7.4 - 7.6 at the testing stations (this is due to additives as water is very soft with a natural pH ~6) ... so for the first time in ages, I looked at the water out of my kitchen tap - still measuring pH 6 - 6.4 (relief

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